In 1972 he interviewed Marc Bolan, who at that time was at the height of his fame as a teen idol and king of glam rock. During the interview Harty asked Bolan what he thought he would be doing when he was forty or sixty years old, Bolan replying that he didn't think he would live that long.
In 1972 he was given his own series, Russell Harty Plus conducting lengthy celebrity interviews, on ITV, which placed him against the BBC's Parkinson. Parts of Russell Harty's interview with the Who in 1973 were included in Jeff Stein's 1979 film The Kids Are Alright, providing notable moments, such as Pete Townshend and Keith Moon ripping off each other's shirt sleeves. In 1975, he interviewed Alice Cooper, French singer Claude François and was one of the first to acknowledge the fact that the Paul Anka song "My Way" was based on a French song of Claude's called "Comme d'habitude". He would also interview François again in 1977.